adjective
a word that describes or modifies a noun or pronoun. In this case, 'unallied' describes something that is not allied or connected.
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The two countries remained unallied in their diplomatic relations.
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The groups were unallied and did not work together on any projects.
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I heard they're unallied now, so don't bring up their past issues.
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Her mind and heart seemed unallied, unable to come to a decision.